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Title Design and evaluation of heat transfer fluids for direct immersion cooling of electronic systems
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Date Accessioned
Degree PhD
Discipline/Department Chemical Engineering
Degree Level doctoral
University/Publisher Georgia Tech
Abstract Comprehensive molecular design was used to identify new heat transfer fluids for direct immersion phase change cooling of electronic systems. Four group contribution methods for thermophysical properties relevant to heat transfer were critically evaluated and new group contributions were regressed for organosilicon compounds. 52 new heat transfer fluids were identified via computer-aided molecular design and figure of merit analysis. Among these 52 fluids, 9 fluids were selected for experimental evaluation and their thermophysical properties were experimentally measured to validate the group contribution estimates. Two of the 9 fluids (C6H11F3 and C5H6F6O) were synthesized in this work. Pool boiling experiments showed that the new fluids identified in this work have superior heat transfer properties than existing coolant HFE 7200. The radiative forcing and global warming potential of new fluids, calculated via a new group contribution method developed in this work and FT-IR analysis, were found to be significantly lower than those of current coolants. The approach of increasing the thermal conductivity of heat transfer fluids by dispersing nanoparticles was also investigated. A model for the thermal conductivity of nanoparticle dispersions (nanofluids) was developed that incorporates the effect of size on the intrinsic thermal conductivity of nanoparticles. The model was successfully applied to a variety of nanoparticle-fluid systems. Rheological properties of nanofluids were also investigated and it was concluded that the addition of nanoparticles to heat transfer fluids may not be beneficial for electronics cooling due to significantly larger increase in viscosity relative to increase in thermal conductivity.
Subjects/Keywords Phonons; Group contribution; Computer-aided molecular design; Heat transfer; Coolant; Electronics cooling; Global warming potential; Nanofluids; Heat Transmission; Heat-transfer media; Fluids Thermal properties
Contributors Teja, Amyn (Committee Chair); Hess, Dennis (Committee Member); Joshi, Yogendra (Committee Member); Liotta, Charles (Committee Member); Realff, Matthew (Committee Member)
Country of Publication us
Record ID handle:1853/44871
Repository gatech
Date Indexed 2018-01-11
Issued Date 2012-07-02 00:00:00
Note [degree] PhD; [advisor] Committee Chair: Teja, Amyn; Committee Member: Hess, Dennis; Committee Member: Joshi, Yogendra; Committee Member: Liotta, Charles; Committee Member: Realff, Matthew;

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